Fractional photo-current dependence of graphene quantum dots prepared from carbon nanotubes
Title | Fractional photo-current dependence of graphene quantum dots prepared from carbon nanotubes |
Publication Type | Journal Article |
Year of Publication | 2015 |
Authors | Kundu, S, Ghosh, S, Fralaide, M, Narayanan, TN, Pillai, VK, Talapatra, S |
Journal | Physical Chemistry Chemical Physics |
Volume | 17 |
Issue | 38 |
Pagination | 24566-24569 |
Date Published | AUG |
ISSN | 1463-9076 |
Abstract | We report on the photo-conductivity studies of chemically synthesized graphene quantum dots (GQDs) of average size 12 nm obtained by the oxidative acid treatment of MWCNTs. The dependence of photocurrent I-ph (I-ph = I-ill - I-dark) on the laser intensity P under a wide range of laser intensities (5 mW <= P <= 60 mW) shows a fractional power dependence of I-ph on light intensity. The temperature dependence (300 K < T < 50 K) of I-ph observed in thin films of these GQDs indicates that in the higher temperature region (T > similar to 100 K), as the temperature increases, the number of thermally generated carriers increase resulting in increased I-ph. At sufficiently low temperatures (T <= 100 K), a constant I-ph is observed, indicating a constant photocarrier density. Such a behavior is typically observed in many photoactive disordered semiconductors, which are often used in a variety of applications. We believe that the investigations presented here will enhance our understanding of the photocurrent generation phenomenon in chemically obtained GQDs. |
DOI | 10.1039/c5cp03306c |
Type of Journal (Indian or Foreign) | Foreign |
Impact Factor (IF) | 4.449 |