Development of unified correlations for volumetric mass-transfer coefficient and effective interfacial area in bubble column reactors for various gas-liquid systems using support vector regression

TitleDevelopment of unified correlations for volumetric mass-transfer coefficient and effective interfacial area in bubble column reactors for various gas-liquid systems using support vector regression
Publication TypeJournal Article
Year of Publication2009
AuthorsGandhi, AB, Gupta, PP, Joshi, JB, Jayaraman, VK, Kulkarni, BD
JournalIndustrial & Engineering Chemistry Research
Volume48
Issue9
Pagination4216-4236
Date PublishedMAY
ISSN0888-5885
Abstract

The objective of this study was to develop a unified correlation for the volumetric mass-transfer coefficient (k(L)a) and effective interfacial area (a) in bubble columns for various gas-liquid systems using support vector regression (SVR-) based modeling technique. From the data published in the open literature, 1600 data points from 27 open sources spanning the years 1965-2007 for k(L)a and 1330 data points from 28 open sources spanning the years 1968-2007 for a were collected. Generalized SVR-based models were developed for the relationship between k(L)a (and a) and each design and operating parameters such as column and sparger geometry, gas-liquid physical properties, operating temperature, pressure, superficial gas velocity, and so on. Further, these models for k(L)a and a are available online at http://www.esnips.com/web/UICT-NCL. The proposed generalized SVR-based correlations for k(L)a and a have prediction accuracies of 99.08% and 98.6% and average absolute relative errors (AAREs) of 7.12% and 5.01%, respectively. Also, the SVR-based correlation provided much improved predictions compared to those obtained using empirical correlations from the literature.

DOI10.1021/ie8003489
Type of Journal (Indian or Foreign)Foreign
Impact Factor (IF)2.071
Divison category: 
Chemical Engineering & Process Development